tranquilize vs unruffle

tranquilize

verb
  • To calm (a person or animal) or put them to sleep using a tranquilizer dart. 

  • To make (something or someone) tranquil. 

unruffle

verb
  • To calm or soothe (a person). 

  • To calm down. 

  • To remove ruffles from; to make smooth. 

How often have the words tranquilize and unruffle occurred in a corpus of books? (source: Google Ngram Viewer )